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Measurements of the structure of turbulent premixed and stratified methane/air flames


Type

Thesis

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Authors

Sweeney, Mark 

Abstract

The influence of stratification on the structure of turbulent methane/air combustion is investigated using experimental data from laboratory scale burners: a weakly turbulent slot burner, and a higher turbulence co-annular swirl burner. The degree of stratification can be controlled independently of the overall fuel/air flow rate. The resulting measurements of scalar and velocity fields provide detailed test cases for existing and emerging turbulent flame models, covering a range of u'/sL from 1 to 10, turbulence intensities from 5% to 60%, and stratification ratios from 1 to 3.

Simultaneous Rayleigh/Raman/CO-LIF measurements of temperature and major species concentrations - CH4, CO2, CO, H2, H2O and O2 - along a line are used to investigate the structure of a series of flames in both the slot and swirl burners. Concurrent cross-planar OH-PLIF allows thermal gradients to be angle corrected to their three-dimensional values. Finally, non-reacting and reacting velocity fields complete the flame database.

The behavior of major species concentrations in the slot and swirl burner with respect to temperature is found to agree well on the mean with unstrained premixed laminar flame calculations. Scalar means conditioned on stoichiometry also show good agreement, aside from hydrogen which is enhanced under stratified conditions. Surface density function and scalar dissipation are lower than calculated values in all cases, suggesting that turbulence-induced thickening dominates the effect of increased strain.

Metrics commonly used to derive flame surface density (FSD) were investigated. FSD may be determined using a statistical method based on measurements of temperature and its gradient, or a geometric method based on 2D temperature or LIF imaging. A third metric, an extension of the geometric method, is proposed. Good agreement is observed between the three metrics.

The current database provides the first detailed high resolution scalar measurements for premixed and stratified flames. The data analysis provides insight into the physics of stratification: for the flames considered, the effects of stratification appear to be surprisingly small compared to those of turbulence, even at significant stratification ratios. The datasets provide a means of validating current and future computational turbulent combustion models.

Description

Date

Advisors

Keywords

Combustion, Stratified, Swirl burner, Slot burner, Weaky turbulent, Turbulent, Laser diagnostics, PIV, PLIF, Flame surface density, FSD, Scalar dissipation rate, Surface density function, Flame thickness, Differential diffusion

Qualification

Doctor of Philosophy (PhD)

Awarding Institution

University of Cambridge
Sponsorship
Work at Sandia National Laboratories was supported by the United States Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences [contract DE-AC04-94-AL85000].